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[<0B640A2B0AC90C24088E053D09EE0D14072503770BA403700837038B07F4034D0A3A0B8B0370034B0394>5<027B09EE0D14>]TJ 0.017 Tc -0.017 Tw T* [<0017>-237<039B0F3B034D0394035C0371037403910393>17<027A05A4091B0B480CCB0683039E03E703AF029403E703770B640A2B>]TJ 0 Tc 0 Tw T* [<0AC90C24088E053D035503D603EF03BB03EF06100F76053C>191<02A20014001702C602A3>191<0370027A>500<0B4804B00683039E03E703AF0294>]TJ 0 -1.677 TD <03E703770B640A2B0AC90C24088E053D0355>Tj 9.3 0 3.3849 9.3 143.8531 354.4616 Tm <0055>Tj 4.65 0 0 9.3 148.9688 354.4616 Tm <02B5>Tj 9.3 0 0 9.3 153.6189 354.4616 Tm [<03D203BD03E7039E03E703AF029403E706100F76053C>500<02A20019001302C602A3>]TJ -10.117 -1.677 Td <037009290F700F9103580B610A52035E03950368027B>Tj 0.024 Tc -0.024 Tw 27.089 35.226 Td [<027903870368056602910378>24<027A063B0CF30A510D11049008A0039B>-232<002F>24<000D>24<0030>]TJ 0 Tc 0 Tw 4.65 0 0 9.3 464.4377 666.4617 Tm <02B5>Tj 0.024 Tc -0.024 Tw 9.3 0 0 9.3 469.3106 666.4617 Tm <03A903E8029403C40F3708DC0370>Tj 0.056 Tc -0.056 Tw -16.974 -1.677 Td [<0C8B0CD60360036803A003E603B403A203DC08680B2E>-215<0018>-215<039B09EE0D1403710360036F0F3B034D>46<027A0A23088E>]TJ 0.051 Tc -0.051 Tw 0 -1.677 TD <03A003B903D303E903D603C703E7039B0A2B0AC909210F300B2E0371036203940B4804B00683039E03E703AF0294>Tj 0.05 Tc -0.05 Tw T* [<03E7>-10<0377>-10<088E053D037403910394039E03E703C303CE03C507F90A52037709EE0D140725039B05890D4303600368>]TJ 0 Tc 0 Tw -0.5 -1.677 Td [<02A2>-20<08DC>-255<001A02A3>]TJ 5.4219 0 0 5.4219 338.1989 608.6323 Tm <0012001102A3>Tj 0.02 Tc -0.02 Tw 9.3 0 0 9.3 346.3318 604.0617 Tm [<027B0E8A09EE0D1407250378>20<027A0E5507F30B120B4804B00683039E03E703AF029403E70369035A>]TJ 0.005 Tc -0.005 Tw -3.75 -1.677 Td [<037003730358>5<027A0B640A2B0AC90C24088E053D035506C3038A036F08140CC9037308B70E710B120B4804B00683039E>]TJ 0 Tc 0 Tw T* <03E703AF029403E70377088E053D0374038B07F4034D05C60A51039B08D403600368027B>Tj 0.053 Tc -0.053 Tw T* [<0279048E09CD03770391034F0374056602910378>53<027A0CA008D703770D430ADD0374062C036E034D03680A83072D>]TJ 0 -1.677 TD [<03740391039304B00FC8037709FD064603A003E603B403A203DC08680B2E09EE0D14039B07F90A520360>53<027A039E>]TJ 0.005 Tc -0.005 Tw 0 -1.677 TD <03E703AF029403E703770B640A2B0AC90C24088E053D03740F1707AE037309EE0D140725037705890D430371057E0F91>Tj T* [<039B094F0376036F03560368>5<027B06DA0B1008680B2E09EE0D14039B0F3B034D0368039E03E703AF029403E703770B64>]TJ 0.023 Tc -0.023 Tw T* [<0A2B0AC90C24088E053D0D530520037406140360036F0378>23<027A>23<0012>23<001A>23<0018>23<0011>-233<0299>-233<0012>23<001A>23<001A>23<0011>-233<0CE50B4503740354035A>]TJ 0.01 Tc -0.01 Tw T* [<036F>1<03E7>1<03C2>1<03C7>1<03A2>1<03DC>1<09EE>1<0D14>1<0C73>1<039B>1<0F3B>1<034D>1<0394>1<0E43>1<0802>1<0355>1<0A3A>1<0FAB>]TJ 0 Tc 0 Tw 5.4219 0 0 5.4219 482.7017 483.8323 Tm <0012001202A3>Tj 0.01 Tc -0.01 Tw 9.3 0 0 9.3 493.6336 479.2617 Tm [<034B>1<036C>1<0368>1<0355>10<027A>]TJ 0.005 Tc -0.005 Tw -19.589 -1.677 Td <09EE0D1405C60A51038D062C08ED03770C260F3B0D63049303770C3A037008EE0F3B0C240371034D03510394038B0377>Tj 0.05 Tc -0.05 Tw T* [<037803730354036C0368>50<027B>50<0013>50<0011>50<0011>50<0011>-213<0CE50B45048E07F10378>50<027A03D003EF03B102940D11049008A0038D061A>]TJ 0.005 Tc -0.005 Tw T* <0BA00AC90DF30AC9060003A703E703D503EF0D11049008A0039B0F170362039408680B2E09EE0D14039B0F3B034D0394>Tj 0 Tc 0 Tw 0 -1.677 TD <0D53052003550E430802035E0395036F034D0394>Tj 5.4219 0 0 5.4219 406.7817 421.4323 Tm <0012001302A3>Tj 9.3 0 0 9.3 414.9146 416.8617 Tm [<027B036003540360027A>4<09EE0D1405730C380A3A027A>4<0D530520>]TJ 0.006 Tc -0.006 Tw -11.125 -1.677 Td [<05390C53>6<027A062C08ED03770C260F3B0D630493>6<027A09EE0D14037708360F620F3B>6<027A0F390D140377060006A50BD0>]TJ 0.005 Tc -0.005 Tw 0 -1.677 TD [<0FE80A510C730377034D036303950377060D0C3A035403920388036F038B>5<027A05660291035505890D430360036809EE>]TJ 0.039 Tc -0.039 Tw T* [<0D14>-221<0014>39<027A>39<0016>-221<038D>-221<0017>-221<039B0F3B>1<034D0394072503550837>1<038B0F0F0395036F034D0394>39<027B>1<03730353>39<027A0771>]TJ 0.006 Tc -0.006 Tw 0 -1.677 TD [<08CC0C3A037009EE0D14>-245<0017>-245<0378>6<027A03620382036F0377039E03E703AF029403E703770B640A2B0AC90C24088E053D>]TJ 0.005 Tc -0.005 Tw 0 -1.677 TD [<09EE0D1403770BA40370083707F4037705C60A51039B0D43077103620394038B03770370034B0393>5<027A056602910377>]TJ ET /PlacedPDF /MC1 BDC /GS0 gs q 1 0 0 1 417.701 753.7594 cm 0 0 m 2.688 -4.263 l 15.477 -3.248 l 17.606 1.725 l 13.445 -2.284 l 4.288 -2.893 l h f Q BT /TT0 1 Tf 0 Tc 0 Tw 8.4 0 0 8.4 170.8446 741.4132 Tm (OH)Tj -3.639 -3.037 Td (secondary alcohol)Tj 2.552 1.004 Td (R)Tj 5.6 0 0 5.6 167.7796 728.1422 Tm (1)Tj 8.4 0 0 8.4 181.3109 724.3395 Tm (R)Tj 5.6 0 0 5.6 187.3773 728.1422 Tm (2)Tj ET 0 0 0 1 K 0.425 w q 1 0 0 1 170.8446 731.8434 cm 0 0 m 3.283 1.743 l S Q q 1 0 0 1 174.1278 739.7711 cm 0 0 m 0 -6.185 l 5.849 -9.378 l S Q BT /TT0 1 Tf 8.4 0 0 8.4 309.4266 742.2067 Tm (O)Tj -0.981 -3.286 Td (ketone)Tj -0.106 1.112 Td (R)Tj 5.6 0 0 5.6 306.3612 727.7448 Tm (1)Tj 8.4 0 0 8.4 319.8934 723.942 Tm (R)Tj 5.6 0 0 5.6 325.9598 727.7448 Tm (2)Tj ET q 1 0 0 1 318.5585 729.9967 cm 0 0 m -5.849 3.59 l -9.133 1.847 l -5.849 3.59 l S Q q 1 0 0 1 311.8895 740.5651 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 313.4501 740.5651 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 203.5194 736.7681 cm 0 0 m 86.791 0 l S Q q 131.337 703.699 332.601 60.948 re W n q 1 0 0 1 289.5467 736.7681 cm 0 0 m -0.932 1.532 l -0.879 1.567 l 1.619 0.574 l 2.489 0.383 3.359 0.191 4.229 0 c 3.359 -0.191 2.489 -0.383 1.619 -0.574 c -0.879 -1.567 l -0.932 -1.541 l h f Q Q BT /TT0 1 Tf 8.4 0 0 8.4 212.9188 741.4117 Tm (catalyst )Tj /TT1 1 Tf (4)Tj /TT0 1 Tf ( )Tj (/)Tj ( )Tj (NaOH)Tj 1.014 -1.834 Td (reflux in H)Tj 5.6 0 0 5.6 259.2533 724.9108 Tm (2)Tj 8.4 0 0 8.4 262.3675 726.0074 Tm (O)Tj -5.327 -1.167 Td (TON up to 320)Tj ET q 1 0 0 1 334.7235 738.2709 cm 0 0 m 3.722 0 l h f Q q 1 0 0 1 334.7235 738.2711 cm 0 0 m 3.722 0 l S Q q 1 0 0 1 336.5856 736.4097 cm 0 0 m 0 3.722 l h f Q q 1 0 0 1 336.5858 736.4097 cm 0 0 m 0 3.722 l S Q BT /TT0 1 Tf 8.4 0 0 8.4 347.867 735.2535 Tm (H)Tj 5.6 0 0 5.6 353.9335 734.1569 Tm (2)Tj 8.4 0 0 8.4 371.3895 734.8336 Tm (\()Tj (5\))Tj ET q 1 0 0 1 394.8514 754.2047 cm 0 0 m 0 -0.708 l S Q [1.411 1.411]0 d q 1 0 0 1 394.8514 752.0846 cm 0 0 m 0 -38.813 l S Q []0 d q 1 0 0 1 394.8514 712.566 cm 0 0 m 0 -0.709 l S Q q 1 0 0 1 426.2762 757.108 cm 0 0 m -8.575 -3.349 l -4.287 -6.241 l 4.87 -5.633 l 9.031 -1.624 l 0 0 l h S Q q 131.337 703.699 332.601 60.948 re W n q 1 0 0 1 432.1356 754.1617 cm 0 0 m 0.091 -1.022 -2.338 -2.072 -5.422 -2.342 c -8.506 -2.611 -11.079 -1.999 -11.17 -0.977 c -11.26 0.049 -8.832 1.1 -5.747 1.367 c -2.663 1.638 -0.09 1.025 0 0 c h S Q Q q 1 0 0 1 425.617 761.5221 cm 0 0 m 0.659 -4.414 l S Q q 1 0 0 1 417.701 753.7594 cm 0 0 m -5.531 0 l S Q q 1 0 0 1 420.6952 749.8522 cm 0 0 m -4.82 -3.959 l S Q q 1 0 0 1 432.62 750.8668 cm 0 0 m 5.937 -3.451 l S Q q 1 0 0 1 435.3075 755.484 cm 0 0 m 5.888 1.878 l S Q q 1 0 0 1 426.2762 748.6002 cm 0 0 m 0.402 -3.736 l S Q BT /TT0 1 Tf 7 0 0 7 425.6629 736.9821 Tm (Ir)Tj 0.335 -1.903 Td (N)Tj -2.026 0.815 Td (O)Tj 3.825 -0.442 Td (O)Tj /TT1 1 Tf 8.4 0 0 8.4 443.827 708.609 Tm (4)Tj ET q 1 0 0 1 424.3036 737.5719 cm 0 0 m -4.327 -3.002 l S Q q 1 0 0 1 428.4969 735.6735 cm 0 0 m 1.148 -4.635 l S Q q 1 0 0 1 417.7694 724.7681 cm 0 0 m -5.916 -4.811 l -4.636 -11.963 l 2.207 -14.699 l 8.255 -9.887 l 7.063 -2.691 l 0 0 l h S Q q 1 0 0 1 413.7518 719.4274 cm 0 0 m 4.281 3.399 l S Q q 1 0 0 1 414.5907 713.9528 cm 0 0 m 5.165 -2.096 l S Q q 1 0 0 1 423.1991 720.9283 cm 0 0 m 1.104 -5.519 l S Q q 1 0 0 1 426.6864 723.6597 cm 0 0 m -1.854 -1.583 l -0.662 -8.778 l 6.269 -11.516 l 12.096 -6.837 l 10.992 0.283 l 7.946 1.859 l S Q q 1 0 0 1 432.5585 713.9528 cm 0 0 m 4.458 3.709 l S Q q 1 0 0 1 437.7772 723.3073 cm 0 0 m 2.771 2.212 l S Q q 1 0 0 1 436.5956 724.5035 cm 0 0 m 2.937 2.428 l S Q 1 J q 1 0 0 1 417.7694 724.7681 cm 0 0 m -0.916 3.769 l S Q EMC /PlacedPDF /MC2 BDC BT /TT2 1 Tf 8.4 0 0 8.4 174.9339 298.8319 Tm (OH)Tj -3.755 -3.037 Td (secondary alcohol)Tj 2.668 1.004 Td (R)Tj 5.6 0 0 5.6 171.8685 285.5604 Tm (1)Tj 8.4 0 0 8.4 185.4002 281.7577 Tm (R)Tj 5.6 0 0 5.6 191.4666 285.5604 Tm (2)Tj ET 0 J q 1 0 0 1 174.9344 289.2626 cm 0 0 m 3.283 1.743 l S Q q 1 0 0 1 178.2176 297.1893 cm 0 0 m 0 -6.184 l 5.848 -9.378 l S Q BT /TT2 1 Tf 8.4 0 0 8.4 326.7591 299.6254 Tm (O)Tj -0.989 -3.286 Td (ketone)Tj -0.098 1.112 Td (R)Tj 5.6 0 0 5.6 323.6936 285.1639 Tm (1)Tj 8.4 0 0 8.4 337.2249 281.3612 Tm (R)Tj 5.6 0 0 5.6 343.2913 285.1639 Tm (2)Tj ET q 1 0 0 1 335.8929 287.4149 cm 0 0 m -5.85 3.591 l -9.133 1.848 l -5.85 3.591 l S Q q 1 0 0 1 329.2229 297.9833 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 330.7845 297.9833 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 207.2112 294.1874 cm 0 0 m 99.143 0 l S Q q 134.452 223.162 334.876 86.589 re W n q 1 0 0 1 305.5911 294.1874 cm 0 0 m -0.932 1.532 l -0.879 1.567 l 1.619 0.574 l 2.489 0.383 3.359 0.191 4.229 0 c 3.359 -0.191 2.489 -0.383 1.619 -0.574 c -0.879 -1.567 l -0.932 -1.541 l h f Q Q BT /TT2 1 Tf 8.4 0 0 8.4 210.5101 298.8309 Tm (water-soluble catalyst )Tj /TT3 1 Tf (5)Tj /TT2 1 Tf 2.007 -1.919 Td (reflux in H)Tj 5.6 0 0 5.6 265.1819 281.6117 Tm (2)Tj 8.4 0 0 8.4 268.2962 282.7089 Tm (O)Tj ET q 1 0 0 1 351.6606 295.2747 cm 0 0 m 3.721 0 l h f Q q 1 0 0 1 351.6604 295.2743 cm 0 0 m 3.722 0 l S Q q 1 0 0 1 353.5227 293.4117 cm 0 0 m 0 3.722 l h f Q q 1 0 0 1 353.5227 293.412 cm 0 0 m 0 3.722 l S Q BT /TT2 1 Tf 8.4 0 0 8.4 363.1185 292.2557 Tm (H)Tj 5.6 0 0 5.6 369.1849 291.1586 Tm (2)Tj 8.4 0 0 8.4 184.0652 243.6805 Tm (OH)Tj -4.202 -1.117 Td (primary alcohol)Tj 2.027 1.004 Td (R)Tj ET q 1 0 0 1 172.8816 248.7831 cm 0 0 m 5.336 3.193 l 11.184 0 l S Q BT /TT2 1 Tf 8.4 0 0 8.4 325.9651 255.1688 Tm (O)Tj -2.986 -3.286 Td (carboxylic acid)Tj 1.899 1.112 Td (R)Tj 2.333 0 Td (OH)Tj ET q 1 0 0 1 335.0999 242.9589 cm 0 0 m -5.85 3.59 l -11.207 0 l -5.85 3.59 l S Q q 1 0 0 1 328.43 253.5272 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 329.9915 253.5272 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 207.2112 248.5819 cm 0 0 m 99.143 0 l S Q q 134.452 223.162 334.876 86.589 re W n q 1 0 0 1 305.5911 248.5819 cm 0 0 m -0.932 1.532 l -0.879 1.566 l 1.619 0.574 l 2.489 0.383 3.359 0.191 4.229 0 c 3.359 -0.191 2.489 -0.383 1.619 -0.574 c -0.879 -1.566 l -0.932 -1.54 l h f Q Q BT /TT2 1 Tf 8.4 0 0 8.4 210.5101 253.2264 Tm (water-soluble catalyst )Tj /TT3 1 Tf (5)Tj /TT2 1 Tf 2.007 -1.919 Td (reflux in H)Tj 5.6 0 0 5.6 265.1819 236.0067 Tm (2)Tj 8.4 0 0 8.4 268.2962 237.1034 Tm (O)Tj ET q 1 0 0 1 351.6606 250.0479 cm 0 0 m 3.721 0 l h f Q q 1 0 0 1 351.6604 250.0477 cm 0 0 m 3.722 0 l S Q q 1 0 0 1 353.5227 248.1858 cm 0 0 m 0 3.722 l h f Q q 1 0 0 1 353.5227 248.1854 cm 0 0 m 0 3.722 l S Q BT /TT2 1 Tf 8.4 0 0 8.4 363.1185 247.0282 Tm (2H)Tj 5.6 0 0 5.6 373.8567 245.9315 Tm (2)Tj 8.4 0 0 8.4 383.0013 291.4218 Tm (\()Tj (6\))Tj 0 -5.313 TD (\()Tj (7\))Tj ET q 1 0 0 1 402.8479 304.3661 cm 0 0 m 0 -0.708 l S Q [1.412 1.412]0 d q 1 0 0 1 402.8479 302.2455 cm 0 0 m 0 -67.078 l S Q []0 d q 1 0 0 1 402.8479 234.4618 cm 0 0 m 0 -0.709 l S Q q 1 0 0 1 425.0384 283.8544 cm 0 0 m 2.42 -3.836 l 13.929 -2.923 l 15.846 1.553 l 12.1 -2.055 l 3.858 -2.604 l h f Q q 1 0 0 1 432.7552 286.869 cm 0 0 m -7.717 -3.015 l -3.858 -5.618 l 4.383 -5.069 l 8.129 -1.462 l 0 0 l h S Q q 134.452 223.162 334.876 86.589 re W n q 1 0 0 1 438.0296 284.2177 cm 0 0 m 0.082 -0.922 -2.103 -1.866 -4.881 -2.107 c -7.656 -2.352 -9.973 -1.8 -10.052 -0.879 c -10.134 0.043 -7.949 0.988 -5.174 1.23 c -2.398 1.473 -0.082 0.923 0 0 c h S Q Q q 1 0 0 1 432.1614 290.8417 cm 0 0 m 0.594 -3.973 l S Q q 1 0 0 1 425.0384 283.8544 cm 0 0 m -4.979 0 l S Q q 1 0 0 1 427.7317 280.3378 cm 0 0 m -4.337 -3.562 l S Q q 1 0 0 1 438.4642 281.2509 cm 0 0 m 5.343 -3.105 l S Q q 1 0 0 1 440.8841 285.4071 cm 0 0 m 5.3 1.689 l S Q q 1 0 0 1 432.4593 278.9969 cm 0 0 m 0.543 -5.367 l S Q q 1 0 0 1 437.5677 271.2411 cm 0 0 m 4.229 0.782 l S Q q 1 0 0 1 431.1761 268.6483 cm 0 0 m -6.062 -3.889 l S Q BT /TT2 1 Tf 7 0 0 7 432.2854 267.6796 Tm (Ir)Tj 0.337 -1.627 Td (N)Tj 1.173 1.986 Td (OH)Tj 4.2 0 0 4.2 453.3548 269.0956 Tm (2)Tj 7 0 0 7 447.0833 258.2089 Tm (OH)Tj /TT3 1 Tf 8.4 0 0 8.4 424.4505 242.7294 Tm (5)Tj ET q 1 0 0 1 434.2825 256.8055 cm 0 0 m -2.309 -1.887 l -1.455 -8.157 l 4.462 -10.748 l 9.644 -6.709 l 8.654 -0.475 l 6.412 0.653 l S Q q 1 0 0 1 429.1761 256.3505 cm 0 0 m 2.798 -1.432 l S Q q 1 0 0 1 433.4212 254.4266 cm 0 0 m 0.62 -4.805 l S Q q 1 0 0 1 438.6546 247.7372 cm 0 0 m 3.732 2.975 l S Q q 1 0 0 1 440.0706 256.3505 cm 0 0 m 1.729 -0.974 l S Q q 1 0 0 1 446.4251 259.2118 cm 0 0 m -3.488 -2.881 l S Q q 1 0 0 1 435.5335 266.9735 cm 0 0 m 1.033 -4.426 l S Q BT /TT2 1 Tf 7 0 0 7 423.0364 254.9188 Tm (N)Tj -1.709 2.072 Td (Me)Tj ET q 1 0 0 1 444.4632 291.4218 cm 0 0 m 7.87 0 l 7.87 -6.534 l S Q BT /TT2 1 Tf 4.2 0 0 4.2 454.0823 287.1425 Tm (2)Tj /C0_1 1 Tf 0.556 -0.022 Td <02B4>Tj /TT2 1 Tf 7 0 0 7 416.4036 263.3856 Tm (N)Tj ET q 1 0 0 1 421.8567 265.3104 cm 0 0 m 3.257 -0.551 l 3.257 -4.467 l S Q q 1 0 0 1 416.4661 262.5477 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394.4835 721.1874 cm 0 0 m 0 -0.709 l S Q q 1 0 0 1 429.5167 759.3563 cm 0 0 m -8.577 -3.349 l -4.288 -6.241 l 4.869 -5.633 l 9.031 -1.624 l 0 0 l h S Q q 132.141 712.789 330.995 54.106 re W n q 1 0 0 1 435.3761 756.411 cm 0 0 m 0.09 -1.024 -2.339 -2.073 -5.424 -2.343 c -8.508 -2.612 -11.08 -2 -11.17 -0.977 c -11.26 0.049 -8.832 1.098 -5.748 1.367 c -2.663 1.637 -0.09 1.025 0 0 c h S Q Q q 1 0 0 1 428.8556 763.7704 cm 0 0 m 0.661 -4.414 l S Q q 1 0 0 1 420.9396 756.0077 cm 0 0 m -5.53 0 l S Q q 1 0 0 1 423.9337 752.1005 cm 0 0 m -4.82 -3.958 l S Q q 1 0 0 1 435.8585 753.1151 cm 0 0 m 5.937 -3.45 l S Q q 1 0 0 1 438.548 757.7323 cm 0 0 m 5.886 1.878 l S Q q 1 0 0 1 429.5167 750.4696 cm 0 0 m 0.709 -4.61 l S Q q 1 0 0 1 434.3361 742.1044 cm 0 0 m 5.582 -0.355 l S Q q 1 0 0 1 433.422 739.0604 cm 0 0 m 2.994 -4.872 l S Q q 1 0 0 1 427.4357 740.5819 cm 0 0 m -4.263 -2.183 l S Q q 1 0 0 1 416.5255 739.3417 cm 0 0 m -2.283 1.999 l -9.184 -0.281 l -10.757 -7.137 l -5.379 -12.206 l 1.648 -9.77 l 2.284 -7.137 l S Q q 1 0 0 1 408.712 737.8934 cm 0 0 m -1.269 -5.125 l S Q q 1 0 0 1 411.6037 728.911 cm 0 0 m 5.024 1.96 l S Q q 1 0 0 1 413.7853 739.4911 cm 0 0 m 1.624 -1.598 l S Q q 1 0 0 1 418.174 729.5721 cm 0 0 m 3.35 -3.502 l S Q BT /TT0 1 Tf 7 0 0 7 428.6974 739.0595 Tm (Ir)Tj -1.661 -0.848 Td (N)Tj 3.459 0.753 Td (Cl)Tj -0.823 -1.511 Td (Cl)Tj -1.97 -1.049 Td (OH)Tj /TT1 1 Tf 8.4 0 0 8.4 435.3644 717.6991 Tm (1)Tj ET EMC /PlacedPDF /MC2 BDC q 1 0 0 1 416.788 284.433 cm 0 0 m 2.689 -4.262 l 15.477 -3.247 l 17.608 1.726 l 13.446 -2.283 l 4.289 -2.892 l h f Q BT /TT2 1 Tf 8.4 0 0 8.4 179.161 278.2542 Tm (OH)Tj -2.954 -3.037 Td (primary and )Tj -1.251 -1.167 Td (secondary alcohol)Tj 3.118 2.171 Td (R)Tj 5.6 0 0 5.6 176.0956 264.9837 Tm (1)Tj 8.4 0 0 8.4 189.6269 261.181 Tm (R)Tj 5.6 0 0 5.6 195.6933 264.9837 Tm (2)Tj ET q 1 0 0 1 179.1601 268.6859 cm 0 0 m 3.283 1.743 l S Q q 1 0 0 1 182.4433 276.6126 cm 0 0 m 0 -6.184 l 5.849 -9.378 l S Q BT /TT2 1 Tf 8.4 0 0 8.4 317.1825 279.0482 Tm (O)Tj -3.862 -3.286 Td (aldehyde and ketone)Tj 2.775 1.112 Td (R)Tj 5.6 0 0 5.6 314.1171 264.5872 Tm (1)Tj 8.4 0 0 8.4 327.6493 260.7845 Tm (R)Tj 5.6 0 0 5.6 333.7157 264.5872 Tm (2)Tj ET q 1 0 0 1 326.3134 266.8382 cm 0 0 m -5.849 3.591 l -9.132 1.848 l -5.849 3.591 l S Q q 1 0 0 1 319.6444 277.4066 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 321.2069 277.4066 cm 0 0 m 0 -7.273 l S Q q 1 0 0 1 203.0956 273.6097 cm 0 0 m 92.838 0 l S Q q 134.899 238.537 325.477 56.785 re W n q 1 0 0 1 295.1708 273.6097 cm 0 0 m -0.932 1.532 l -0.879 1.567 l 1.619 0.574 l 2.489 0.383 3.359 0.191 4.229 0 c 3.359 -0.191 2.489 -0.383 1.619 -0.574 c -0.879 -1.567 l -0.932 -1.541 l h f Q Q BT /TT2 1 Tf 8.4 0 0 8.4 215.5653 278.2533 Tm (catalyst )Tj /TT3 1 Tf (2)Tj /TT2 1 Tf ( )Tj (/)Tj ( )Tj (NaOMe)Tj 0.29 -1.905 Td (reflux in toluene)Tj T* (TON up to 1000)Tj ET q 1 0 0 1 342.765 275.1138 cm 0 0 m 3.721 0 l h f Q q 1 0 0 1 342.7646 275.1136 cm 0 0 m 3.722 0 l S Q q 1 0 0 1 344.6262 273.2526 cm 0 0 m 0 3.721 l h f Q q 1 0 0 1 344.6259 273.2523 cm 0 0 m 0 3.721 l S Q BT /TT2 1 Tf 8.4 0 0 8.4 354.2255 272.0952 Tm (H)Tj 5.6 0 0 5.6 360.2919 270.998 Tm (2)Tj 8.4 0 0 8.4 374.7323 271.6751 Tm (\()Tj (2\))Tj ET q 1 0 0 1 393.9169 286.3118 cm 0 0 m 0 -0.708 l S Q [1.399 1.399]0 d q 1 0 0 1 393.9169 284.2044 cm 0 0 m 0 -32.875 l S Q []0 d q 1 0 0 1 393.9169 250.6302 cm 0 0 m 0 -0.709 l S Q q 1 0 0 1 425.3651 287.7827 cm 0 0 m -8.577 -3.35 l -4.288 -6.241 l 4.869 -5.633 l 9.031 -1.624 l 0 0 l h S Q q 134.899 238.537 325.477 56.785 re W n q 1 0 0 1 431.2245 284.8363 cm 0 0 m 0.09 -1.023 -2.339 -2.073 -5.424 -2.342 c -8.508 -2.612 -11.08 -2 -11.17 -0.976 c -11.26 0.049 -8.832 1.099 -5.748 1.367 c -2.663 1.638 -0.09 1.025 0 0 c h S Q Q q 1 0 0 1 424.704 292.1967 cm 0 0 m 0.661 -4.414 l S Q q 1 0 0 1 416.788 284.433 cm 0 0 m -5.53 0 l S Q q 1 0 0 1 419.7821 280.5257 cm 0 0 m -4.82 -3.958 l S Q q 1 0 0 1 431.7069 281.5414 cm 0 0 m 5.937 -3.451 l S Q q 1 0 0 1 434.3964 286.1585 cm 0 0 m 5.886 1.877 l S Q q 1 0 0 1 425.3651 279.2738 cm 0 0 m 0.401 -3.736 l S Q q 1 0 0 1 429.8192 271.8529 cm 0 0 m 5.582 -0.355 l S Q q 1 0 0 1 423.2841 270.7659 cm 0 0 m -6.224 -3.088 l S Q BT /TT2 1 Tf 7 0 0 7 424.3983 269.3788 Tm (Ir)Tj 0.032 -1.805 Td (N)Tj 1.656 1.687 Td (Cl)Tj 0.274 -1.687 Td (OH)Tj /TT3 1 Tf 8.4 0 0 8.4 412.3231 246.5462 Tm (2)Tj ET q 1 0 0 1 411.9267 271.4974 cm 0 0 m -5.978 -2.878 l -6.432 -9.147 l -1.429 -12.818 l 4.613 -10.121 l 5.134 -3.819 l 0 0 l h S Q q 1 0 0 1 411.7323 269.7572 cm 0 0 m 3.834 -2.762 l S Q q 1 0 0 1 407.0702 267.9565 cm 0 0 m -0.243 -4.762 l S Q q 1 0 0 1 410.7245 260.2719 cm 0 0 m 4.32 2.078 l S Q q 1 0 0 1 424.2724 258.8743 cm 0 0 m -2.665 -1.331 l -3.217 -7.634 l 1.981 -11.468 l 7.926 -8.673 l 8.339 -2.372 l 6.398 -0.779 l S Q q 1 0 0 1 416.5399 261.3763 cm 0 0 m 5.067 -3.833 l S Q q 1 0 0 1 422.9081 256.7455 cm 0 0 m -0.455 -4.823 l S Q q 1 0 0 1 426.5351 249.0638 cm 0 0 m 4.299 2.079 l S Q q 1 0 0 1 429.8192 257.1537 cm 0 0 m 1.47 -1.333 l S Q q 1 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143.794 334.616 62.964 re W n q 1 0 0 1 305.009 191.1935 cm 0 0 m -0.932 1.532 l -0.879 1.567 l 1.619 0.574 l 2.489 0.383 3.359 0.191 4.229 0 c 3.359 -0.191 2.489 -0.383 1.619 -0.574 c -0.879 -1.567 l -0.932 -1.541 l h f Q Q BT /TT4 1 Tf 8.4 0 0 8.4 213.0012 195.838 Tm (water-soluble catalyst )Tj /TT5 1 Tf (3)Tj /TT4 1 Tf 2.007 -1.919 Td (reflux in H)Tj 5.6 0 0 5.6 267.673 178.6187 Tm (2)Tj 8.4 0 0 8.4 270.7873 179.7159 Tm (O)Tj -5.605 -1.167 Td (TON up to 2550)Tj /TT5 1 Tf -0.943 -1.358 Td (Reusable Aqueous)Tj 0.499 -1.167 Td (Catalytic System)Tj ET q 1 0 0 1 349.533 192.6972 cm 0 0 m 3.722 0 l h f Q q 1 0 0 1 349.5334 192.6974 cm 0 0 m 3.722 0 l S Q q 1 0 0 1 351.396 190.836 cm 0 0 m 0 3.721 l h f Q q 1 0 0 1 351.3957 190.836 cm 0 0 m 0 3.721 l S Q BT /TT4 1 Tf 8.4 0 0 8.4 360.9933 189.6788 Tm (H)Tj 5.6 0 0 5.6 367.0598 188.5816 Tm (2)Tj 8.4 0 0 8.4 381.5012 189.2589 Tm (\(3\))Tj ET q 1 0 0 1 400.0041 197.3995 cm 0 0 m 0 -0.708 l S Q [1.477 1.477]0 d q 1 0 0 1 400.0041 195.214 cm 0 0 m 0 -31.753 l S Q []0 d q 1 0 0 1 400.0041 162.7227 cm 0 0 m 0 -0.709 l S Q q 1 0 0 1 422.1662 193.8224 cm 0 0 m 2.42 -3.837 l 13.93 -2.923 l 15.846 1.553 l 12.1 -2.055 l 3.858 -2.604 l h f Q q 1 0 0 1 429.884 196.837 cm 0 0 m -7.718 -3.015 l -3.859 -5.618 l 4.382 -5.069 l 8.128 -1.462 l 0 0 l h S Q q 130.33 143.794 334.616 62.964 re W n q 1 0 0 1 435.1574 194.1856 cm 0 0 m 0.082 -0.922 -2.103 -1.866 -4.879 -2.108 c -7.656 -2.352 -9.972 -1.801 -10.052 -0.879 c -10.134 0.043 -7.948 0.988 -5.173 1.23 c -2.396 1.473 -0.08 0.923 0 0 c h S Q Q q 1 0 0 1 429.2912 200.8097 cm 0 0 m 0.593 -3.973 l S Q q 1 0 0 1 422.1662 193.8224 cm 0 0 m -4.979 0 l S Q q 1 0 0 1 424.8615 190.3058 cm 0 0 m -4.338 -3.563 l S Q q 1 0 0 1 435.5939 191.2188 cm 0 0 m 5.342 -3.106 l S Q q 1 0 0 1 438.0119 195.3751 cm 0 0 m 5.3 1.689 l S Q q 1 0 0 1 429.5881 188.9649 cm 0 0 m 0.501 -3.967 l S Q q 1 0 0 1 434.298 182.6065 cm 0 0 m 4.266 0.991 l S Q q 1 0 0 1 427.7629 180.1602 cm 0 0 m -3.112 -1.545 l S Q BT /TT4 1 Tf 7 0 0 7 428.8762 178.7726 Tm (Ir)Tj 0.233 -1.301 Td (N)Tj 1.354 1.604 Td (OH)Tj 4.2 0 0 4.2 450.4846 179.7945 Tm (2)Tj 7 0 0 7 442.7023 171.4073 Tm (OH)Tj /TT5 1 Tf 8.4 0 0 8.4 420.3556 156.7628 Tm (3)Tj ET q 1 0 0 1 418.6652 177.9903 cm 0 0 m -3.157 1.397 l -8.351 -2.728 l -7.409 -8.94 l -1.72 -11.418 l 3.578 -7.45 l 3.175 -4.599 l S Q q 1 0 0 1 415.7043 177.6495 cm 0 0 m 2.395 -1.017 l S Q q 1 0 0 1 411.5549 174.8624 cm 0 0 m 0.814 -4.694 l S Q q 1 0 0 1 416.8137 168.1768 cm 0 0 m 3.756 2.98 l S Q q 1 0 0 1 430.1486 170.1827 cm 0 0 m -2.307 -1.887 l -1.454 -8.156 l 4.462 -10.747 l 9.644 -6.709 l 8.655 -0.475 l 6.412 0.653 l S Q q 1 0 0 1 422.2433 170.5401 cm 0 0 m 5.599 -2.244 l S Q q 1 0 0 1 429.2873 167.8038 cm 0 0 m 0.62 -4.804 l S Q q 1 0 0 1 434.5207 161.1143 cm 0 0 m 3.732 2.975 l S Q q 1 0 0 1 435.9367 169.7276 cm 0 0 m 1.729 -0.974 l S Q q 1 0 0 1 442.2931 172.589 cm 0 0 m -3.489 -2.881 l S Q q 1 0 0 1 431.9142 178.1143 cm 0 0 m 0.287 -2.345 l S Q BT /TT4 1 Tf 7 0 0 7 419.0119 173.797 Tm (N)Tj -1.699 1.4 Td (HO)Tj ET q 1 0 0 1 415.508 179.3878 cm 0 0 m 0 2.927 l S Q q 1 0 0 1 440.548 201.3897 cm 0 0 m 7.87 0 l 7.87 -6.534 l S Q BT /TT4 1 Tf 4.2 0 0 4.2 450.1672 197.1104 Tm (2)Tj /C0_1 1 Tf 0.556 -0.022 Td <02B4>Tj ET EMC /PlacedPDF /MC4 BDC BT /TT6 1 Tf 8.4 0 0 8.4 359.9292 97.557 Tm (O)Tj -2.651 -3.999 Td (lactone)Tj -15.882 3.918 Td (OH)Tj -1.834 -3.918 Td (diol)Tj ET 0.512 w q 1 0 0 1 223.5898 87.807 cm 0 0 m 97.875 0 l S Q q 1 0 0 1 320.5459 87.807 cm 0 0 m -1.122 1.844 l -1.06 1.886 l 1.948 0.691 l 5.092 0 l 1.948 -0.691 l -1.06 -1.886 l -1.122 -1.854 l h f Q BT /TT6 1 Tf 8.4 0 0 8.4 229.0996 92.451 Tm (water-soluble catalyst )Tj /TT7 1 Tf (3)Tj /TT6 1 Tf 2.007 -1.919 Td (reflux in H)Tj 5.6 0 0 5.6 283.77 75.2328 Tm (2)Tj 8.4 0 0 8.4 286.8843 76.3294 Tm (O)Tj ET q 1 0 0 1 370.9476 87.066 cm 0 0 m 3.722 0 l h f Q 0.425 w q 1 0 0 1 370.9473 87.0657 cm 0 0 m 3.723 0 l S Q q 1 0 0 1 372.8106 85.2039 cm 0 0 m 0 3.721 l h f Q q 1 0 0 1 372.8105 85.2035 cm 0 0 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